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Browsing by Subject "Molecular vibrations"

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    • Article  

      The Active Site Structure of Heme a3 3+-C≡N-CuB2+ of Cytochrome aa 3 Oxidase as Revealed from Resonance Raman Scattering 

      Pinakoulaki, Eftychia; Vamvouka, M.; Varotsis, Constantinos (2003)
      Resonance Raman and FTIR spectroscopies have been employed to investigate the structure of the heme a3-C≡N-CuB complex of oxidized cytochrome aa3 oxidase. The characterization of this complex is essential since a central ...

    • Article  

      Femtosecond UV pump/near-IR probe studies of the solvent-dependent excited-state decay dynamics of chlorine dioxide 

      Hayes, Sophia C.; Cooksey, C. C.; Wallace, P. M.; Reid, P. J. (2001)
      The excited-state decay and geminate-recombination dynamics of chlorine dioxide (OClO) are investigated using UV pump/near-IR probe spectroscopy. Experiments are performed with 200-fs time resolution on OClO dissolved in ...

    • Article  

      Fourier transform infrared evidence for a ferric six-coordinate nitrosylheme b3 complex of cytochrome cbb3 oxidase from Pseudomonas stutzeri at ambient temperature 

      Stavrakis, Stavros; Pinakoulaki, Eftychia; Urbani, A.; Varotsis, Constantinos (2002)
      We report the first vibrational study of NO bound to an oxidized heme-copper oxidase. Cytochrome cbb3 oxidase from P. stutzeri reduces both O2 and NO to H2O and N2O, respectively. The ferric nitrosyl complex of cbb3 exhibits ...

    • Article  

      Inelastic electron tunneling erases coupling-pathway interferences 

      Skourtis, Spiros S.; Waldeck, D. H.; Beratan, David N. (2004)
      Theoretical analysis of nonadiabatic electron-transfer reactions in molecules usually assumes that electron amplitude propagates coherently from the reductant to the oxidant via covalent and noncovalent coupling pathways. ...

    • Article  

      The production and decay kinetics of CIOO in water and freon-11: A time-resolved resonance Raman study 

      Hayes, Sophia C.; Thomsen, C. L.; Reid, P. J. (2001)
      The production and decay kinetics of ClOO in water and freon-11 were studied using time-resolved resonance Raman (TRRR) spectroscopy. The formation of ClOO following OClO photoexcitation at 390 nm was investigated using ...

    • Article  

      Time resolved infrared absorption studies of geminate recombination and vibrational relaxation in OCIO photochemistry 

      Bolinger, J. C.; Hayes, Sophia C.; Reid, P. J. (2004)
      The first ultrafast time-resolved infrared absorption studies of the geminate recombination and vibrational relaxation dynamics of aqueous chlorine dioxide (OCIO) were presented. The rapid increase in optical density ...

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